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Libra Compatibility with All 12 Zodiac Signs Best to WorstLibra heart perfect zodiac signs are twins, aquarius, and aries. When it comes to matters of the heart, Libra seeks harmony and understanding above all else. The Twins can provide adventure and joy to the connection, while The Water Bearer shares Libra's appreciation for intellect and originality. Aries, known for their fire, can ignite a spark in Libra's spirit. Libra and these signs create a well-rounded and rewarding union.